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MoS₂ HER stability is allotrope-dependent: lamellar MoS₂ degrades under open circuit conditions, while amorphous MoS₃ₓ loses sulfur during HER, generating undercoordinated Mo sites. Simultaneous ICP-MS

Heads up — this abstract doesn’t match the title. The title references acetaldehyde detection in CO reduction on Cu, but the abstract is about a

A tetraalkylsulfonamide (TAS) additive displaces water from the Zn²⁺ solvation shell, suppressing HER by an order of magnitude and eliminating dendrite and passivation layer formation.

Size-selected Au nanoparticles peak in CO selectivity at ~3 nm, reaching 60% faradaic efficiency at low overpotentials. HRTEM identifies multiply twinned particles as the favourable

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Allotrope-dependent activity-stability relationships of molybdenum sulfide hydrogen evolution electrocatalysts

MoS₂ HER stability is allotrope-dependent: lamellar MoS₂ degrades under open circuit conditions, while amorphous MoS₃ₓ loses sulfur during HER, generating undercoordinated Mo sites. Simultaneous ICP-MS and EC-MS monitoring of dissolution products underpins revised stability metrics and a proposed HER mechanism accounting for both Mo and S dissolution pathways.

April 29, 2024

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